Quantum entanglement is a fascinating phenomenon that forms the basis of many quantum technologies. Recently, scientists from the National University of Singapore (NUS) have made significant strides in enhancing the efficiency of generating entangled photon pairs through excitonic interactions in non-linear optical crystals. This groundbreaking research has the potential to revolutionize the field of quantum optics and light sources.

Entangled photons, which are particles of light, exhibit a unique connection where the properties of two quantum particles are interdependent, regardless of the distance between them. To create entangled photons, a process known as spontaneous parametric down-conversion (SPDC) is typically used by shining light on non-linear optical crystals. However, the efficiency of SPDC has been a limiting factor in generating entangled photon pairs.

The research team at NUS, led by Associate Professor Su Ying Quek, has discovered that harnessing many-body excitonic interactions in non-linear optical crystals can significantly enhance the efficiency of SPDC. Excitonic interactions involve the interaction between negative and positive charges that are formed when light interacts with the crystal, creating pairs known as excitons. The proximity of these charges plays a crucial role in increasing the efficiency of SPDC, depending on the energy or frequency of the light.

The team’s research findings, published in Physical Review Letters, highlight the importance of excitonic effects in improving the efficiency of generating entangled photon pairs. Through fully quantum mechanical calculations, the team demonstrated that the interaction between negative and positive charges can lead to a substantial increase in SPDC efficiency. This effect was particularly evident when compared to conventional treatments that neglect excitonic interactions.

By utilizing ultrathin crystals, the research team was able to overcome technical challenges associated with SPDC, such as the phase matching problem. Despite the belief that ultrathin crystals may reduce efficiency due to their smaller volume, the stronger excitonic interactions in these crystals actually alleviate this issue. This breakthrough makes ultrathin crystals a promising source for producing entangled photons in a more efficient manner.

The team’s theoretical approach, applied to NbOI2, a layered non-linear optical material, not only improved SPDC efficiency but also shed light on second harmonic generation (SHG). The team found that excitonic enhancement is particularly pronounced when the frequency of the “pump” beam aligns closely with an excitation frequency in the crystal. Furthermore, matching one of the entangled photon’s frequencies with another excitation frequency in the crystal can further enhance SPDC efficiency.

Overall, the research conducted by the NUS team opens up exciting possibilities for the future of quantum-photonic technologies. By leveraging excitonic interactions in non-linear optical crystals, the efficiency of generating entangled photon pairs can be significantly enhanced, paving the way for more practical applications in quantum communication and quantum computing. This research showcases the immense potential of ultrathin materials in advancing quantum light sources and building hybrid quantum-photonic platforms for next-generation devices.

Science

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